hmm you have missed like a year or two then (the Haruhi movie came out last year in DVD/BR if I'm not wrong but probably it was shown in japanese theaters earlier like many films do before their year-later home releases over there), there have been many great series, movies and OVAs between 2010-2011, of course is up to you what genres and other aspects you like or you're interested to watch... for me these ones are my favorites which I suggest you:
Kamisama Dolls
No. 6
Gosick
Fate/Stay Night - Unlimited Blade Works
Evangelion 2.22 You Can(not) Advance (after Evangelion 1.11)
Yumekui Merry
Fractale
Psychological, Life or Death challenges:
Kaiji Season 2 (obviously after you watch S1)
Deadman Wonderland
Gore and monsters:
Hellsing Ultimate VII and VIII (if you haven't watched from I to VI yet do it right now)
Blade
Kore wa Zombie desu ka
Superheroes:
Tiger & Bunny
X-Men
Wolverine
Saint Seiya The Lost Canvas
Slice of life, drama and/or romance:
Usagi Drop
Kimi ni Todoke S2
Colorful (the movie, not the ecchi series of the same name from many years ago)
Anohana
Yosuga no Sora
Sports:
Redline
Tailenders
Ecchi, weird situations and/or comedy in general:
Mawaru Penguindrum
Koe de Oshigoto The Animation
KissxSis
Higurashi no Naku Koro ni Kira
Carnival Phantasm
Nichijou
Mayo Chiki
Working!!
Onii-chan no Koto Nanka Zenzen Suki Janain Dakara ne!!
Dororon Enma-kun
Level E